论文标题

纳米装饰物中的高$ q $ quasi-bic状态的多极第二谐波一代

Multipolar second-harmonic generation from high-$Q$ quasi-BIC states in nanoresonators

论文作者

Volkovskaya, Irina I., Xu, Lei, Huang, Lujun, Smirnov, Alexander I., Miroshnichenko, Andrey

论文摘要

多模干扰和多极相互作用控制光学纳米孔子和非线性纳米ant的功能。最近,已经预测,在单个亚波长介电颗粒中的高质量超级腔模式(准BIC态)的激发已被预测可以提高纳米级的非线性频率转换。在这里,我们提出了多极模型,该模型捕获了由纳米孔子中这样的高$ Q $模式驱动的线性和非线性响应背后的物理。我们表明,可以通过耦合的泄漏模式的多极变化来理解藻类纳米风格中准BIC状态的形成。特别是,杂交轴向对称的Te偏振模式可以看作是多物的叠加,其基础主要由磁性偶极子和八杆构成。参数空间中的准BIC点出现在完全抑制偶极损耗的地方。与该状态的有效光耦合通过方位角极化光束照明实现,与其多极了。我们在标准的非遗传耦合模式理论与多极模型之间建立了一对一的对应关系,该模型可以透明地解释散射特征。使用我们的方法,我们从藻类纳米风险中得出了生成的第二谐辐射的多极组成,并使用全波数值模拟验证它。在泵耗尽的耦合非线性模型中考虑了第二谐音辐射到基本频率上的反作用。提出了一种杂交金属含量纳米坦纳,以提高转化效率高于数百分之百分之的,并实现非线性参数下调。我们的发现描述了在非线性纳米素化应用功能元素设计中的深入概念框架和新颖的有前途的策略。

Multimode interference and multipolar interplay govern functionalities of optical nanoresonators and nonlinear nanoantennas. Recently, excitation of the high-quality supercavity modes (quasi-BIC states) in individual subwavelength dielectric particles has been predicted to boost the nonlinear frequency conversion at the nanoscale. Here, we put forward the multipolar model which captures the physics behind linear and nonlinear response driven by such high-$Q$ modes in nanoresonators. We show that formation of the quasi-BIC state in the AlGaAs nanodisk can be understood through multipolar transformations of coupled leaky modes. In particular, the hybridized axially symmetric TE-polarized modes can be viewed as superpositions of multipoles, with a basis of parent multipoles constituted mainly by magnetic dipoles and octupole. The quasi-BIC point in the parameter space appears where dipolar losses are totally suppressed. The efficient optical coupling to this state is implemented via azimuthally polarized beam illumination matching its multipolar origin. We establish a one-to-one correspondence between the standard non Hermitian coupled-mode theory and multipolar models that enables transparent interpretation of scattering characteristics. Using our approach, we derive the multipolar composition of the generated second-harmonic radiation from the AlGaAs nanodisk and validate it with full-wave numerical simulations. Back-action of the second-harmonic radiation onto the fundamental frequency is taken into account in the coupled nonlinear model with pump depletion. A hybrid metal-dielectric nanoantenna is proposed to augment the conversion efficiency up to tens of per cent and actualize the nonlinear parametric downconversion. Our findings delineate the in-depth conceptual framework and novel promising strategies in the design of functional elements for nonlinear nanophotonics applications.

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