论文标题

核转变的直接激光激发理论

The theory of direct laser excitation of nuclear transitions

论文作者

von der Wense, Lars, Bilous, Pavlo V., Seiferle, Benedict, Stellmer, Simon, Weitenberg, Johannes, Thirolf, Peter G., Pálffy, Adriana, Kazakov, Georgy

论文摘要

提出了基于密度矩阵形式主义的核状态的直接激光激发的全面理论研究。核时钟异构体$^{229 \ text {m}} $ th进行了详细讨论,因为它可以使用现有技术直接激发激发,并为这项工作提供动力。光学BLOCH方程是为纯核两级系统的最简单情况得出的,并且考虑到磁性子园的存在,超细结构和Zeeman在外部场中的分裂。分别讨论了在固态环境中以自由原子和离子以及核的核水平分裂。根据获得的方程,审查了低饱和限制中的核群转移。此外,还考虑了核兔振荡,功率扩展和核双光子激发。最后,该理论应用于$^{229 \ text {m}} $ th和$^{235 \ text {m}} $ u的特殊情况,是最低的激发能量的核激发态。该论文的目的是进行教学审查,并明确给出许多计算。

A comprehensive theoretical study of direct laser excitation of a nuclear state based on the density matrix formalism is presented. The nuclear clock isomer $^{229\text{m}}$Th is discussed in detail, as it could allow for direct laser excitation using existing technology and provides the motivation for this work. The optical Bloch equations are derived for the simplest case of a pure nuclear two-level system and for the more complex cases taking into account the presence of magnetic sub-states, hyperfine-structure and Zeeman splitting in external fields. Nuclear level splitting for free atoms and ions as well as for nuclei in a solid-state environment is discussed individually. Based on the obtained equations, nuclear population transfer in the low-saturation limit is reviewed. Further, nuclear Rabi oscillations, power broadening and nuclear two-photon excitation are considered. Finally, the theory is applied to the special cases of $^{229\text{m}}$Th and $^{235\text{m}}$U, being the nuclear excited states of lowest known excitation energies. The paper aims to be a didactic review with many calculations given explicitly.

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