论文标题

表面粗糙度在纳米纳语等离子系统中的影响

Impact of surface roughness in nanogap plasmonic systems

论文作者

Ciracì, Cristian, Vidal-Codina, Ferran, Yoo, Daehan, Peraire, Jaime, Oh, Sang-Hyun, Smith, David R.

论文摘要

最近的结果表明,在两个金属元件之间对分离距离的距离进行了前所未有的控制,这是数百个纳米大小的尺寸的基础,这是自由电子非局部响应的影响。但是,由于制造引起的表面粗糙度,大多数金属系统仍然遭受一定程度的不均匀性。这种系统中的纳米级粗糙度可能会阻碍对微观相互作用的作用的理解。在这里,我们研究了表面粗糙度在中红外频率下共鸣的同轴纳米剂中的影响。我们表明,尽管随机粗糙度以不可预测的方式改变了共振,但仍然可以清楚地观察到非局部效应的影响。粗糙度引起的系统峰值扰动与单个样品的有效间隙大小有很强的相关性。然后,由于制造缺陷而引起的波动可以通过对结构集合进行测量来抑制,在该结构集合中,在大量样品上平均提供了对理想系统光学特性的精确度量。

Recent results have shown unprecedented control over separation distances between two metallic elements hundreds of nanometers in size, underlying the effects of free-electron nonlocal response also at mid-infrared wavelengths. Most of metallic systems however, still suffer from some degree of inhomogeneity due to fabrication-induced surface roughness. Nanoscale roughness in such systems might hinder the understanding of the role of microscopic interactions. Here we investigate the effect of surface roughness in coaxial nanoapertures resonating at mid-infrared frequencies. We show that although random roughness shifts the resonances in an unpredictable way, the impact of nonlocal effects can still be clearly observed. Roughness-induced perturbation on the peak resonance of the system shows a strong correlation with the effective gap size of the individual samples. Fluctuations due to fabrication imperfections then can be suppressed by performing measurements on structure ensembles in which averaging over a large number of samples provides a precise measure of the ideal system's optical properties.

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