论文标题

石墨烯中狄拉克龙超快动力学的第一原理研究

First-principles study of ultrafast dynamics of Dirac plasmon in graphene

论文作者

Novko, Dino

论文摘要

探索低损坏的二维等离子体模式被认为是在等离子科学和技术中实现纳米级的光操作的核心。在这种情况下,泵探针光谱是研究这些集体模式和相应的能量传递过程的强大工具。在这里,我介绍了一项关于石墨烯中非平衡狄拉克门的第一原理研究,其中仍未完全探索在超快条件下的阻尼通道。用电子孔对浓度的热增加来解释了激光诱导的等离子能的蓝光。有趣的是,虽然平衡石墨烯等离子体的阻尼途径完全由用声音子散射统治,但光诱导的等离子主要将其能量转移到强耦合的热光学声子上,这解释了实验性观察到的等离子体线路的实验性提高的提高。本研究为新型二维系统和异质结构中等离子体时间动力学的深入理解铺平了道路。

Exploring low-loss two-dimensional plasmon modes is considered central for achieving light manipulation at the nanoscale and applications in plasmonic science and technology. In this context, pump-probe spectroscopy is a powerful tool for investigating these collective modes and the corresponding energy transfer processes. Here, I present a first-principles study on non-equilibrium Dirac plasmon in graphene, wherein damping channels under ultrafast conditions are still not fully explored. The laser-induced blueshift of plasmon energy is explained in terms of thermal increase of the electron-hole pair concentration in the intraband channel. Interestingly, while damping pathways of the equilibrium graphene plasmon are entirely ruled by scatterings with acoustic phonons, the photoinduced plasmon predominantly transfers its energy to the strongly coupled hot optical phonons, which explains the experimentally-observed tenfold increase of the plasmon linewidth. The present study paves the way for an in-depth theoretical comprehension of plasmon temporal dynamics in novel two-dimensional systems and heterostructures.

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