论文标题

使用分子固体作为缩放码头

Using Molecular Solids as Scaled-up Qubits

论文作者

Roberts, Malcolm P.

论文摘要

提出的扩大量子位是分子,它们在非常低的温度下显示出较大的振幅运动,而矩阵捕获了它们。这些包括离子固体,例如四苯甲酸铵(ATPB)或Xenon基质中的甲烷稀释。以这种方式,从启动开始就存在巨大的数字。每种量子都具有多种感兴趣的转变,这些量子使用(不需要外部田地,超低温度或超高真空条件),使用各种良好的实验技术,范围为10至3300 cm-1。详细描述的是ATPB中的过渡。其中包括:(i)铵离子量子标准的IR N-H非对称振动,几乎可以在四苯基硼酸酯基质内自由旋转其C3轴。这会导致多级振动取向,即使在前三个方向水平之间的核自旋冻结引起的核自旋冻结,也表现出多个带。方向水平和控制问题间距离之间的无障碍隧道频率使该量子置于多种实验设置中同时产生大型纠缠和稳定的叠加的强大候选者; (ii)拉曼允许四苯基硼酸酯阴离子值的正常模式。这些是从非常低的温度到300 K的实验解决的。检查了进一步的量子示例和感兴趣的过渡。具有多晶阵列的实验设置,无论是在给定还是几个位置,都可以使用这种方法。

The scaled-up qubits proposed are molecules which display large amplitude motions at very low temperatures and the matrix that traps them. These comprise ionic solids such as ammonium tetraphenylborate (ATPB) or methane dilute in a xenon matrix. In this manner, an enormous number qubits are present from inception. Each kind of qubit has a multiplicity of transitions of interest which are observed (without the need of external fields, ultra-low temperatures or ultra-high vacuum conditions) using diverse well established experimental techniques at frequencies ranging from 10 to 3300 cm-1. Described in detail are the transitions in ATPB. These include: (i) the IR N-H asymmetric vibration of the ammonium ion qubit which nearly freely rotate about their C3 axes inside the tetraphenylborate matrix. This results in a multi-level vibration-orientation which exhibits multiple bands even at very low temperatures due to nuclear spin freezing between the first three orientation levels. Accessible tunneling frequencies between the orientation levels and the possibility to control inter-qubit distance make this qubit a strong candidate to generate concurrently large entanglement and stable superposition in diverse experimental set-ups; and (ii) the Raman allowed normal modes of the tetraphenylborate anion qubit. These are experimentally resolved from very low temperatures up to 300 K. Further qubit examples and transitions of interest are examined. Experimental setups with multi-crystal arrays, both in a given or several locations, become possible using this approach.

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