论文标题

CA $ _ {2} $ ruo $ _ {4} $的当前引起的相位共存的证据及其对磁性顺序的影响

Evidence for current-induced phase coexistence in Ca$_{2}$RuO$_{4}$ and its influence on magnetic order

论文作者

Jenni, K., Wirth, F., Dietrich, K., Berger, L., Sidis, Y., Kunkemöller, S., Grams, C. P., Khomskii, D. I., Hemberger, J., Braden, M.

论文摘要

与X射线和中子衍射实验相结合的准和时间分辨的传输测量结果,我们研究了在纯净的CA $ _2 $ _4 $ _4 $中在当前密度应用下出现的非平衡状态。对电流引起的开关的时间分辨研究发现了缓慢的电导弛豫,可以通过加热来识别,并且可以明确证明一种固有机制的速度。电流诱导的相变导致复杂的衍射模式。分离的Bragg反射可以通过其晶格参数与金属和绝缘阶段相关联,这表明具有相共存的真实结构,与温度和电流强度有很大变化。在冷却时,在金属和绝缘阶段之间的$ C $晶格常数的第三个贡献。在低电流密度下,此额外阶段的出现在$ \ sim $ 100 K以下,并伴随着抑制抗磁性顺序,否则该抗通过当前的携带状态可以共存。讨论了中间阶段的可能起源。

Combining quasistatic and time-resolved transport measurements with X-ray and neutron diffraction experiments we study the non-equilibrium states that arise in pure and in Ti substituted Ca$_2$RuO$_4$ under the application of current densities. Time-resolved studies of the current-induced switching find a slow conductance relaxation that can be identified with heating and a fast one that unambiguously proves an intrinsic mechanism. The current-induced phase transition leads to complex diffraction patterns. Separated Bragg reflections that can be associated with the metallic and insulating phases by their lattice parameters, indicate a real structure with phase coexistence that strongly varies with temperature and current strength. A third contribution with a $c$ lattice constant in between those of metallic and insulating phases appears upon cooling. At low current densities, this additional phase appears below $\sim$100 K and is accompanied by a suppression of the antiferromagnetic order that otherwise can coexist with current carrying states. A possible origin of the intermediate phase is discussed.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源