论文标题
使用多色光场的大型糖蜜样冷却力用于分子:理论描述
Large molasses-like cooling forces for molecules using polychromatic optical fields: A theoretical description
论文作者
论文摘要
最近的理论研究表明,在具有不同成分,几何形状和对称性的复杂多原子分子中,快速光学循环应是可行的。但是,随着复合分子质量的增长,使用激光光限制和局限分子束所需数量的光子散射事件也是如此。利用光场和分子之间的相干动量交换可以抑制自发的发射,并显着降低减速和捕获的实验复杂性。我们与BAH作为测试物种合作,已经确定了一种可靠的,实验性的可行构型,以使用$ x-a $和$ x-b $电子过渡的多色光场获得类似糖蜜的冷却力。使用时间依赖性密度矩阵以及蒙特卡洛模拟的数值解,我们证明,具有较大捕获速度的抑制排放速率(超级)糖蜜($ \ sim 40 $ m/s)通常对于具有光学循环中心的增长复杂性的多原子分子通常是可行的。预计所提出的超级糖蜜不仅将量子控制扩展到具有丰富振动衰变通道的新分子物种,而且还显着增加了以前激光冷却的diatomic和triotomic物种的捕获密度。
Recent theoretical investigations have indicated that rapid optical cycling should be feasible in complex polyatomic molecules with diverse constituents, geometries and symmetries. However, as a composite molecular mass grows, so does the required number of photon scattering events necessary to decelerate and confine molecular beams using laser light. Utilizing coherent momentum exchange between light fields and molecules can suppress spontaneous emission and significantly reduce experimental complexity for slowing and trapping. Working with BaH as a test species, we have identified a robust, experimentally viable configuration to achieve large molasses-like cooling forces for molecules using polychromatic optical fields addressing both $X-A$ and $X-B$ electronic transitions, simultaneously. Using numerical solutions of the time-dependent density matrix as well as Monte Carlo simulations, we demonstrate that creation of Suppressed Emission Rate (SupER) molasses with large capture velocities ($\sim 40$ m/s) is generically feasible for polyatomic molecules of increasing complexity that have an optical cycling center. Proposed SupER molasses are anticipated to not only extend quantum control to novel molecular species with abundant vibrational decay channels, but also significantly increase trapped densities for previously laser-cooled diatomic and triatomic species.