论文标题

在统一的相对论电子光束非弹性散射的统一描述中,桥接纳米镜和凝结物质形式主义

Bridging nano-optics and condensed matter formalisms in a unified description of inelastic scattering of relativistic electron beams

论文作者

Lourenço-Martins, Hugo, Lubk, Axel, Kociak, Mathieu

论文摘要

在过去的几十年中,电子能量损失光谱(EELS)领域中实验突破的开花触发了各种理论发展。这些必须处理完全不同的情况,从原子分辨的声子映射到通过表面等离子体映射经过的电子圆二色性。尽管早期尝试这样做,但他们都依靠非常不同的物理近似,并且尚未和解。为了朝这个方向努力,我们报告了快速电子非弹性散射的标量相对论量子电动力学(QED)方法的发展。可以将该理论适应以描述所有现代鳗鱼实验,并且在相关的近似值下,可以简化为最后的鳗鱼理论。在这个目标中,我们在本文中介绍了与电子非弹性散射相关的标量相对论Q的基础知识。然后,我们在两个曾经对鳗鱼的拮抗剂描述(通常用于描述光子激发)和准静态混合动力外形(MDFF)之间给出了明确的关系,更适合描述材料的核心电子激发。然后,我们使用该理论建立两个重要的鳗鱼相关方程。第一个将空间解析的鳗鱼与光子传播器的假想部分以及传入和外发电子束波函数联系起来,合成用于分析空间解析的鳗鱼实验的最常见理论。第二个表明,电子束密度矩阵的演变与相互的相干张量成正比,证明靶标的电磁相关性在探测电子束的相干性能中印在目标中。

In the last decades, the blossoming of experimental breakthroughs in the domain of electron energy loss spectroscopy (EELS) has triggered a variety of theoretical developments. Those have to deal with completely different situations, from atomically resolved phonon mapping to electron circular dichroism passing by surface plasmon mapping. All of them rely on very different physical approximations and have not yet been reconciled, despite early attempts to do so. As an effort in that direction, we report on the development of a scalar relativistic quantum electrodynamic (QED) approach of the inelastic scattering of fast electrons. This theory can be adapted to describe all modern EELS experiments, and under the relevant approximations, can be reduced to any of the last EELS theories. In that aim, we present in this paper the state of the art and the basics of scalar relativistic QED relevant to the electron inelastic scattering. We then give a clear relation between the two once antagonist descriptions of the EELS, the retarded green Dyadic, usually applied to describe photonic excitations and the quasi-static mixed dynamic form factor (MDFF), more adapted to describe core electronic excitations of material. We then use this theory to establish two important EELS-related equations. The first one relates the spatially resolved EELS to the imaginary part of the photon propagator and the incoming and outgoing electron beam wavefunction, synthesizing the most common theories developed for analyzing spatially resolved EELS experiments. The second one shows that the evolution of the electron beam density matrix is proportional to the mutual coherence tensor, proving that quite universally, the electromagnetic correlations in the target are imprinted in the coherence properties of the probing electron beam.

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