论文标题
X射线自由电子激光器的自我引用的原位到达时间监视器
A self-referenced in-situ arrival time monitor for X-ray free-electron lasers
论文作者
论文摘要
我们提出了一种新型,高度用途和自我引用的到达时间监视器,用于测量从自由电子激光器的硬X射线脉冲与光学激光脉冲之间的飞秒时间延迟,该脉冲直接在用于泵送实验的同一样品上测量。两次chi鼠和皮秒长的光学光学超级脉冲脉冲以970 fs的相互固定时间延迟横穿样品,而飞秒X射线脉冲在两种脉冲之间的瞬间都达到了一个瞬间。在样品后面,在没有X射线脉冲的情况下,超紧张脉冲在时间上重叠,以产生接近完美的破坏性干扰。用X射线脉冲刺激样品在某些光学波长下提供非零贡献,这是X射线脉冲的相对到达时间的度量,其精度高于25 fs。我们发现,我们的监视器与SACLA XFEL的现有计时诊断的出色共识,Pearson相关值为0.98。我们证明了高灵敏度对低至30 $μ$ J的X射线脉冲测量X射线脉冲。使用自由流动的液体射流作为相互作用样品,可确保每个X射线/光学事件的样品体积的完整替换,从而使其实用程序即使以MHz的重复率XFEL源也可以实现。
We present a novel, highly versatile, and self-referenced arrival time monitor for measuring the femtosecond time delay between a hard X-ray pulse from a free-electron laser and an optical laser pulse, measured directly on the same sample used for pump-probe experiments. Two chirped and picosecond long optical supercontinuum pulses traverse the sample with a mutually fixed time delay of 970 fs, while a femtosecond X-ray pulse arrives at an instant in between both pulses. Behind the sample the supercontinuum pulses are temporally overlapped to yield near-perfect destructive interference in the absence of the X-ray pulse. Stimulation of the sample with an X-ray pulse delivers non-zero contributions at certain optical wavelengths, which serve as a measure of the relative arrival time of the X-ray pulse with an accuracy of better than 25 fs. We find an excellent agreement of our monitor with the existing timing diagnostics at the SACLA XFEL with a Pearson correlation value of 0.98. We demonstrate a high sensitivity to measure X-ray pulses with pulse energies as low as 30 $μ$J. Using a free-flowing liquid jet as interaction sample ensures the full replacement of the sample volume for each X-ray/optical event, thus enabling its utility even at MHz repetition rate XFEL sources.