论文标题

X射线自由电子激光器的自我引用的原位到达时间监视器

A self-referenced in-situ arrival time monitor for X-ray free-electron lasers

论文作者

Diez, Michael, Galler, Andreas, Schulz, Sebastian, Boemer, Christina, Coffee, Ryan N., Hartmann, Nick, Heider, Rupert, Wagner, Martin S., Helml, Wolfram, Katayama, Tetsuo, Sato, Tokushi, Sato, Takahiro, Yabashi, Makina, Bressler, Christian

论文摘要

我们提出了一种新型,高度用途和自我引用的到达时间监视器,用于测量从自由电子激光器的硬X射线脉冲与光学激光脉冲之间的飞秒时间延迟,该脉冲直接在用于泵送实验的同一样品上测量。两次chi鼠和皮秒长的光学光学超级脉冲脉冲以970 fs的相互固定时间延迟横穿样品,而飞秒X射线脉冲在两种脉冲之间的瞬间都达到了一个瞬间。在样品后面,在没有X射线脉冲的情况下,超紧张脉冲在时间上重叠,以产生接近完美的破坏性干扰。用X射线脉冲刺激样品在某些光学波长下提供非零贡献,这是X射线脉冲的相对到达时间的度量,其精度高于25 fs。我们发现,我们的监视器与SACLA XFEL的现有计时诊断的出色共识,Pearson相关值为0.98。我们证明了高灵敏度对低至30 $μ$ J的X射线脉冲测量X射线脉冲。使用自由流动的液体射流作为相互作用样品,可确保每个X射线/光学事件的样品体积的完整替换,从而使其实用程序即使以MHz的重复率XFEL源也可以实现。

We present a novel, highly versatile, and self-referenced arrival time monitor for measuring the femtosecond time delay between a hard X-ray pulse from a free-electron laser and an optical laser pulse, measured directly on the same sample used for pump-probe experiments. Two chirped and picosecond long optical supercontinuum pulses traverse the sample with a mutually fixed time delay of 970 fs, while a femtosecond X-ray pulse arrives at an instant in between both pulses. Behind the sample the supercontinuum pulses are temporally overlapped to yield near-perfect destructive interference in the absence of the X-ray pulse. Stimulation of the sample with an X-ray pulse delivers non-zero contributions at certain optical wavelengths, which serve as a measure of the relative arrival time of the X-ray pulse with an accuracy of better than 25 fs. We find an excellent agreement of our monitor with the existing timing diagnostics at the SACLA XFEL with a Pearson correlation value of 0.98. We demonstrate a high sensitivity to measure X-ray pulses with pulse energies as low as 30 $μ$J. Using a free-flowing liquid jet as interaction sample ensures the full replacement of the sample volume for each X-ray/optical event, thus enabling its utility even at MHz repetition rate XFEL sources.

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