论文标题

二维材料中的激子trion-polariton

Exciton-Trion-Polaritons in Two-Dimensional Materials

论文作者

Rana, Farhan, Koksal, Okan, Jung, Minwoo, Shvets, Gennady, Vamivakas, A. Nick, Manolatou, Christina

论文摘要

我们为掺杂的二维材料中的激子 - trion-polariton提供了多体理论。激子 - trion-Polaritons是涉及激子,TRIONS和PHOTON的强大相干杂交激发。这些极化子的签名最近在实验中出现。在这些极性子中,两体激子状态通过激子 - photon相互作用耦合到材料基态,并通过库仑相互作用将4体TRION状态耦合到激子状态。 TRION状态未直接将其与材料基态耦合。这些偏振子的能量摩孔分散体展示了三个频段。我们使用Green的功能来计算不同掺杂密度下极性子的能量带分散体和偏振子的组成。极化带之间的能量分裂以及北极频带的光谱重量取决于激发器与激子之间的库仑耦合的强度,这又取决于掺杂密度。激子与绑定和未结合的Trion状态耦合。后者是激子 - 电子散射状态,其包含对于捕获偏振子带之间的光谱重量转移是掺杂密度的函数所必需的。

We present a many-body theory for exciton-trion-polaritons in doped two-dimensional materials. Exciton-trion-polaritons are robust coherent hybrid excitations involving excitons, trions, and photons. Signatures of these polaritons have been recently seen in experiments. In these polaritons, the 2-body exciton states are coupled to the material ground state via exciton-photon interaction and the 4-body trion states are coupled to the exciton states via Coulomb interaction. The trion states are not directly optically coupled to the material ground state. The energy-momentum dispersion of these polaritons exhibit three bands. We calculate the energy band dispersions and the compositions of polaritons at different doping densities using Green's functions. The energy splittings between the polariton bands, as well as the spectral weights of the polariton bands, depend on the strength of the Coulomb coupling between the excitons and the trions and which in turn depends on the doping density. The excitons are Coulomb coupled to both bound and unbound trion states. The latter are exciton-electron scattering states and their inclusion is necessary to capture the spectral weight transfer among the polariton bands as a function of the doping density.

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