论文标题

使用短波长种子的自由电子激光研究超快狂犬动力学

Studying ultrafast Rabi dynamics with a short-wavelength seeded free-electron laser

论文作者

Nandi, Saikat, Olofsson, Edvin, Bertolino, Mattias, Carlström, Stefanos, Zapata, Felipe, Busto, David, Callegari, Carlo, Di Fraia, Michele, Eng-Johnsson, Per, Feifel, Raimund, Gallician, Guillaume, Gisselbrecht, Mathieu, Maclot, Sylvain, Neoričić, Lana, Peschel, Jasper, Plekan, Oksana, Prince, Kevin C., Squibb, Richard J., Zhong, Shiyang, Demekhin, Philipp V., Meyer, Michael, Miron, Catalin, Badano, Laura, Danailov, Miltcho B., Giannessi, Luca, Manfredda, Michele, Sottocorona, Filippo, Zangrando, Marco, Dahlström, Jan Marcus

论文摘要

Rabi振荡是与随时间变化的领域相互作用的两级系统中种群的定期调制。它们在物理学中无处不在,在不同地区的应用,例如光子学,纳米电子,电子显微镜和量子信息。虽然Rabi开发的理论旨在用于旋转磁场的费米子,但Autler和Townes意识到它也可以用来描述旋转波近似中的相干光物质相互作用\ cite。尽管已经使用了十多年的强烈纳米波长光源,但在如此短的波长下,尚未直接观察到Rabi动力学。在这里,我们表明,来自种子的自由电子激光器的飞秒极端硫酸脉冲可以驱动基态和氦原子中激发态之间的拉比振荡。测得的光发射信号揭示了Autler-Townes Doublet以及避免的横断,这都是量子光学元件的商标。使用超出强场上近似的理论分析,我们发现双重结构的超快堆积是从谐振和非谐振光电离途径之间的量子干扰效应遵循的。鉴于最近有强烈的Attosecond和几秒钟的极端极度脉冲脉冲,我们的结果提供了使用自由电子激光器在短波长下进行相干过程的超快操纵的机会。

Rabi oscillations are periodic modulations of populations in two-level systems interacting with a time-varying field. They are ubiquitous in physics with applications in different areas such as photonics, nano-electronics, electron microscopy, and quantum information. While the theory developed by Rabi was intended for fermions in gyrating magnetic fields, Autler and Townes realized that it could also be used to describe coherent light-matter interaction within the rotating wave approximation\cite. Although intense nanometer-wavelength light-sources have been available for more than a decade, Rabi dynamics at such short wavelengths have not been observed directly. Here we show that femtosecond extreme-ultraviolet pulses from a seeded free-electron laser can drive Rabi oscillations between the ground state and an excited state in helium atoms. The measured photoemission signal revealed an Autler-Townes doublet as well as an avoided crossing, phenomena that are both trademarks of quantum optics. Using theoretical analyses that go beyond the strong-field approximation, we found that the ultrafast build-up of the doublet structure follows from a quantum interference effect between resonant and non-resonant photoionization pathways. Given the recent availability of intense attosecond and few-femtosecond extreme-ultraviolet pulses, our results offer opportunities to carry out ultrafast manipulation of coherent processes at short wavelengths using free-electron lasers.

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