论文标题

高压下非中心对称RE6HF超导体的超导和结构特性

Superconducting and structural properties of non-centrosymmetric Re6Hf superconductor under high pressure

论文作者

Mariappan, Sathiskumar, Krishnan, Manikandan, Bhoi, Dilip, Ma, Hanming, Gouchi, Jun, Singh, R. P., Motla, Kapil, Vajeeston, Ponniah, Sonachalam, Arumugam, Uwatoko, Yoshiya

论文摘要

我们报告了高压对多晶非中心对称超导体RE6HF的超导,涡旋固定和结构特性的影响。超导过渡温度TC显示出适度的减小,随着压力P的增加,随着斜率-0.046 k/gpa(-0.065 k/gpa),从电阻率测量最高8 GPA(磁性测量测量〜1.1 GPA)估计。最高约18 GPA的结构分析揭示了晶格常数的单调降低,而无需进行任何结构过渡和较高的大量模量B0 = 333.63 GPA,表明结构的稳定性。此外,在绝对温度(HC2(0)&HC1(0))下,上临界场和下部临界场从周围的压力值略有下降,因为压力增加到2.5 GPA。此外,使用涡流的热活化通量流达到P〜2.5 GPA,显示了涡旋的激活能的双线性场依赖性,从而证实了单个和集体固定涡流状态的共存。此外,使用集体固定理论对临界电流密度的分析表明,随着压力的增加,ΔTC向ΔL固定的转化可能是由于晶界的迁移。此外,使用密度功能理论的频带结构计算表明,状态的密度随压力而适度降低,这可能是压力下TC降低如此小的原因。

We report the effect of high pressure on the superconducting, vortex pinning, and structural properties of a polycrystalline non-centrosymmetric superconductor Re6Hf. The superconducting transition temperature, Tc, reveals a modest decrease as pressure P increases with a slope -0.046 K/GPa (-0.065 K/GPa) estimated from resistivity measurements up to 8 GPa (magnetization measurement ~ 1.1 GPa). Structural analysis up to ~18 GPa reveals monotonic decreases of lattice constant without undergoing any structural transition and a high value of bulk modulus B0= 333.63 GPa, indicating the stability of the structure. Furthermore, the upper critical field and lower critical field at absolute temperature (Hc2(0) & Hc1(0)) decreases slightly from the ambient pressure value as pressure increases up to 2.5 GPa. In addition, up to P ~ 2.5 GPa using thermally activated flux flow of vortices revealed a double linearity field dependence of activation energy of vortices, confirming the coexistence of single and collective pinning vortex states. Moreover, analysis of critical current density using the collective pinning theory showed the transformation of δTc to δl pinning as pressure increases, possibly due to migration of grain boundaries. Besides, the band structure calculations using density functional theory show that density of states decreases modestly with pressure, which may be a possible reason for such a small decrease in Tc by pressure.

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