论文标题

精确控制并通过放松振荡器来运行和停止化学反应

Accurate control to run and stop chemical reactions via relaxation oscillators

论文作者

Shi, Xiaopeng, Gao, Chuanhou, Dochain, Denis

论文摘要

多个反应模块的调节在分子计算和通过化学反应构建深度学习网络中非常普遍,而对于该模块的顺序执行总是与化学反应的本质平行性质相对的头痛。精确切换多个反应模块在开发和关闭中,是编程化学反应系统中的核心作用。与设置物理隔室或添加人类干预信号不同,我们基于放松振荡来采用化学振荡器的概念,并将相应的时钟信号组件分配到需要调节的模块中。本文主要在三个模块的调节任务下证明了振荡器的设计过程,并为自动终止模块周期提供了合适的方法。我们在普通微分方程的水平上提供了模拟结果,并确保方程可以转化为相应的化学反应网络。

Regulation of multiple reaction modules is quite common in molecular computation and deep learning networks construction through chemical reactions, as is always a headache for that sequential execution of modules goes against the intrinsically parallel nature of chemical reactions. Precisely switching multiple reaction modules both on and off acts as the core role in programming chemical reaction systems. Unlike setting up physical compartments or adding human intervention signals, we adopt the idea of chemical oscillators based on relaxation oscillation, and assign corresponding clock signal components into the modules that need to be regulated. This paper mainly demonstrates the design process of oscillators under the regulation task of three modules, and provides a suitable approach for automatic termination of the modules cycle. We provide the simulation results at the level of ordinary differential equation and ensure that equations can be translated into corresponding chemical reaction networks.

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